Dissertations, Theses, and Capstone Projects

Date of Degree

2-2024

Document Type

Dissertation

Degree Name

Ph.D.

Program

Chemistry

Advisor

Rein V. Ulijn

Committee Members

Mateusz Marianski

Sharon Loverde

Ruth Stark

Subject Categories

Biochemistry | Biology and Biomimetic Materials | Biomaterials | Computational Chemistry | Materials Chemistry | Physical Chemistry | Polymer and Organic Materials

Keywords

Supramolecular, Self-Assembly, Peptides, Molecular Dynamics, Bioinspired, Minimalistic

Abstract

The challenge of establishing a sustainable and circular economy for materials in medicine and technology necessitates bioinspired design. Nature's intricate machinery, forged through evolution, relies on a finite set of biomolecular building blocks with through-bond and through-space interactions. Repurposing these molecular building blocks requires a seamless integration of computational modeling, design, and experimental validation. The tools and concepts developed in this thesis pioneer new directions in peptide-materials design, grounded in fundamental principles of physical chemistry. We present a synergistic approach that integrates experimental designs and computational methods, specifically molecular dynamics simulations, to gain in-depth molecular insights crucial for advancing the design of sustainable, bio-inspired (nano)technology for both biological and materials applications.

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